By R. Goulard (auth.), Marshall Lapp, C. M. Penney (eds.)
The Laser Raman Workshop at the r"eas urement of gasoline Properti es i sone of aseries of occasional conferences equipped in a casual workshop structure throughout the stimulation of venture SQUID, workplace of Naval examine. This workshop is the second one to be equipped on gas-phase purposes of Raman scattering. either Raman workshops have been supported by means of venture SQUID, ONR, and the Air strength Aero Propulsion Laboratory, Wright-Patterson Air strength Base. the 1st Raman Workshop used to be held on the AVCO Everett learn Laboratory, Everett, Massachusetts, with their co-sponsorship in January 1972 less than the chairmanship of D. A. Leonard. the current assembly used to be co-sponsored by means of the overall electrical examine and improvement middle, and held at their facility in Schenectady, long island. we're thankful to venture SQUID, AFAPL, and GE for his or her beneficiant monetary aid of this Workshop, and to undertaking SQUID for underwriting the ebook expenditures of the court cases. As is usually the case for winning conferences, many folks contributed considerably to the association and execution of this workshop. Professor Robert Goulard supported, aided, and inspired us within the so much necessary methods, and we're indebted to him. We obtained extra precious help and the aid of Dr. Ralph Roberts, Director, and Mr. James R. Patton, Jr., of the ability department, workplace of Naval study; from Dr. William H. Heiser, leader Scientist of the Aero Propulsion Laboratory; and from Dr. James M.
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L for the trace scattering. From the fundamental expressions (ga) and (9b), it is easy to derive the intensities of the observed components as functions of I tr and I anis . when different optical arrangements are involved. 111. THE DIFFERENT RAMAN BAND TYPES We shall briefly diseuss now the different band types for each sort of molecular rotator. In what fol1ows, we assume that the lower vibrational level is always totally symmetrie. A. Linear Molecules The rotational spectral terms are given by F(J) = BJ(J+l)- Di(J+1)2, (10) where Band D are rotational constants; B is proportional to the reeiprocal of the inertia moment and D aceounts for the eentrifugal effect.
The frequeney of the band origin is 'U vvib 'U 'U vexe . - b,v vib and the Raman frequeneies referred to the band origin are b,';J = '0'Ram - '0'vib = exi J(J+1) . (20) We emphasize here the meaning of our notation: the b,~Ram are the usual Raman shifts, while the b,~ are the frequeneies referredto the band origin. In the Stokes speetrum, their variations are of opposite signs. The intensities of the lines, for traee and anisotropy seattering (see Ref. 2), are I tr . (J) er I anis . (J) Usua lly, C Ctr .
5. R. Gaufres and S. Sportouch, J. Mol. Spectry. 39, 527 (1971). 6. J. Herranz and B. P. Stoicheff, J. Mol. Spectry. lQ, 448 (1963). 7. M. Lapp, L. M. Goldman and C. M. Penney, Science 8. F. N. Masri and N. H. Fletcher, J. Chem. Phys. 52,5759,(970). 9. S. Sportouch and R. Gaufres, J. Chim. Phys. 69, 470 (1972). 10. 175, 1112 (1972). S. Sportouch, C. Lacoste and R. Gaufres, J. Mol. Struct. ~, 119 (1971). R. GAUFRES 41 11. R. Gaufres and S. Sportouch, Compt. Rend. Acad. Sei. Paris 995 (1972). 272, 12.